Abstract

Micropatterns based on the oriented nanowires have attracted research interests for their unique physicochemical advantages in various applications of electric microdevices. Here, we proposed a facile fibrous dewetting strategy by spreading and dewetting of the silver nanowire (AgNW) solution on the vertical aligned carbon nanotube array (ACNTs) for preparing multidimensional aligned nanowires array, based on the elastocapillary coalescence. The unidirectional shrinking of the liquid film on the top of ACNTs happens during the dewetting process, as a result of the elastocapillary coalescence of ACNTs, which drives the AgNWs aligned along normal direction of liquid film shrinkage on the top of ACNTs. Thus, a multidimensional aligned NWs array was prepared, composing of the horizontally oriented NWs of top layer and vertical ACNT bundles of under layer connected by CNT yarns. A bendable flexible electrode was prepared using the as-prepared multidimensional aligned nanowires array, showing high stability during bending cycles (1800 cycles). Moreover, the multidimensional aligned nanowires array is also applicable for fabricating strain sensors, which show stable resistance response under strain. We envision that the as-developed approach shed new light on easy manufacture NW-based micropatterns.

Highlights

  • The nanowires-based micropatterns have provided vast opportunities for their unique physicochemical advantages in developing various photoelectric devices, including piezoelectric devices [1], sensing [2], light-emitting diodes [3], supercapacitors [4,5], and electronic skin [6,7]

  • ACNTswere weretransferred transferredfrom fromglass glasssubstrates substratestotoflexible flexiblesubstrate substrate(PET, (PET, PDMS), lead- to

  • We demonstrated a strain sensor using the as-developed multidimensional aligned NWs array, as Figure 4 illustrates

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Summary

Introduction

The nanowires-based micropatterns have provided vast opportunities for their unique physicochemical advantages in developing various photoelectric devices, including piezoelectric devices [1], sensing [2], light-emitting diodes [3], supercapacitors [4,5], and electronic skin [6,7]. Various solution-coating techniques have been developed for aligning 1D nanomaterials due for their merits of mild conditions and large-area preparation, such as printing [18], microfluidic approaches [19], rod coating [20,21], Langmuir–Blodgett [22,23,24,25], blade-coating [26,27], and solution shearing technique [28,29] These techniques suffer from complex for samples pretreatment process, uncontrolled deposition and aggregation of NWs during the film formation process, which remains a barrier for preparing the highly integrated devices. The essence of 1D nanomaterials arrangement is to introduce directional force during the film formation process, forcing

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