Abstract

We apply the time-dependent R-matrix method to investigate harmonic generation from Ne(+) at a wavelength of 390 nm and intensities up to 10(15) Wcm(-2). The 1s(2)2s(2)2p(4) (3)P(e), (1)D(e), and (1)S(e) states of Ne(2+) are included as residual-ion states to assess the influence of interference between photoionization channels associated with these thresholds. The harmonic spectrum is well approximated by calculations in which only the (3)P(e) and (1)D(e) thresholds are taken into account, but no satisfactory spectrum is obtained when a single threshold is taken into account. Within the harmonic plateau, extending to about 100 eV, individual harmonics can be suppressed at particular intensities when all Ne(2+) thresholds are taken into account. The suppression is not observed when only a single threshold is accounted for. Since the suppression is dependent on intensity, it may be difficult to observe experimentally.

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