Abstract
We present several new materials made of acceptor units (TCNQ and [Ni(dmit) 2]) and stilbazolium-based chromophores for second-order optical nonlinearity. The subtil adjustement in the redox potentials necessary for: ( i) maintaining the material in a semi-conducting state, to offer a good range of transparency in a broad nearinfrared domain; ( ii) allowing electronic interaction, to promote a pathway towards efficient interplays between the properties is analyzed The possibility of combining both properties on the same entity with the TTF skeleton is also discussed.
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