Monte Carlo simulation of the response of ESR dosimeters added with gadolinium exposed to thermal, epithermal and fast neutrons

Abstract

Monte Carlo numerical calculations of the response of alanine and ammonium tartrate ESR (electron spin resonance) dosimeters exposed to neutron fields with different energy spectra are reported. Results have been obtained for various gadolinium concentrations inside the dosimeters. Furthermore, in order to simulate the in-phantom response we have carried out calculations by varying the depth of the dosimeter. We have found that a large enhancement is obtained for thermal neutrons, because of the very high capture cross section of gadolinium to thermal neutrons. A good enhancement was obtained for epithermal neutrons, whereas the sensitivity improvement in the case of fast neutron irradiation is poor. Furthermore, the simulations carried out by varying the depth suggests that an appreciable sensitivity to thermal and epithermal neutrons could be observed for in-phantom measurements in the 2–3 cm depth range. These results can provide useful insight for future experiments with epithermal neutron beams (such as those used in neutron capture therapy) and for future applications in neutron capture therapy dosimetry.