Abstract

Purpose The purpose of this paper is to investigate the effect of lanthana (La2O3) on the mechanical and tribological properties of polyimide (PI). Design/methodology/approach The mechanical and tribological properties of PI nanocomposites filled with La2O3 were studied by molecular dynamic simulations to explore the deep mechanisms from an atomic or molecular view. Findings The results showed that the hardness of the PI matrix increased after La2O3 modification with a decrease of 72.4% nanoindentation depth. Besides, the friction coefficient of PI decreased by 72.2% after filling La2O3, and the shear deformation was largely reduced under the same conditions. The adsorption effect of La2O3 on the PI molecular, which reduced the atomic relative concentration, velocity, interaction with counterpart Fe layer and the temperature rise in the frictional interface, contributed to the improvement of the mechanical and tribological performance. Originality/value This study reveals the friction and wear mechanism of PI composites filled with rare earth oxide at the nanoscale.

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