Abstract

Graphene, as the thinnest material ever found, exhibits unconventionally relativistic behaviour of Dirac fermions. However, unusual phenomena (such as superconductivity) arise when stacking two graphene layers and twisting the bilayer graphene. The relativistic Dirac fermion in graphene has been widely studied and understood, but the large change observed in twisted bilayer graphene (TBG) is intriguing and still unclear because only van der Waals force (vdW) interlayer interaction is added from graphene to TBG and such a very weak interaction is expected to play a negligible role. To understand such dramatic variation, we studied the electronic structures of monolayer, bilayer and twisted bilayer graphene. Twisted bilayer graphene creates different moiré patterns when turned at different angles. We proposed tight-binding and effective continuum models and thereby drafted a computer code to calculate their electronic structures. Our calculated results show that the electronic structure of twisted bilayer graphene changes significantly even by a tiny twist. When bilayer graphene is twisted at special “magic angles”, flat bands appear. We examined how these flat bands are created, their properties and the relevance to some unconventional physical property such as superconductivity. We conclude that in the nanoscopic scale, similar looking atomic structures can create vastly different electronic structures. Like how P. W. Anderson stated that similar looking fields in science can have differences in his article “More is Different”, similar moiré patterns in twisted bilayer graphene can produce different electronic structures.

Highlights

  • IntroductionSome fascinating phenomena such as superconductivity and other novel strong-correlation properties(Bistritzer & MacDonald, 2011; Cao, Fatemi, Demir, Fang, Tomarken, Luo, Sanchez-Yamagishi, Watanabe, Taniguchi, Kaxiras, Ashoori, & Jarillo-Herrero, 2018; Cao, Fatemi, Fang, Watanabe, Taniguchi, Kaxiras, & Jarillo-Herrero, 2018), which are unconceivable in graphene, are found to arise in twisted bilayer graphene (TBG)

  • In the article (Anderson, 1972), he explained how symmetry is of great importance to physics, objects that appear symmetric may not be symmetric at the quantum scale

  • A tiny change in angle could create a vastly different moiré pattern. Some fascinating phenomena such as superconductivity and other novel strong-correlation properties(Bistritzer & MacDonald, 2011; Cao, Fatemi, Demir, Fang, Tomarken, Luo, Sanchez-Yamagishi, Watanabe, Taniguchi, Kaxiras, Ashoori, & Jarillo-Herrero, 2018; Cao, Fatemi, Fang, Watanabe, Taniguchi, Kaxiras, & Jarillo-Herrero, 2018), which are unconceivable in graphene, are found to arise in TBG. Such a big change observed from graphene to TBG is very intriguing but unclear, because it is very counterintuitive to ascribe such a big change to the tiny change in twist or to the very weak van der Waals force interlayer interaction.To comprehend the huge difference due to tiny change in TBG, we examined the electronic properties of graphene and conventional bilayer graphene, created twisted bilayer graphene and investigated the electronic band structure of TBG within tight binding approximation and effective continuum model

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Summary

Introduction

Some fascinating phenomena such as superconductivity and other novel strong-correlation properties(Bistritzer & MacDonald, 2011; Cao, Fatemi, Demir, Fang, Tomarken, Luo, Sanchez-Yamagishi, Watanabe, Taniguchi, Kaxiras, Ashoori, & Jarillo-Herrero, 2018; Cao, Fatemi, Fang, Watanabe, Taniguchi, Kaxiras, & Jarillo-Herrero, 2018), which are unconceivable in graphene, are found to arise in TBG Such a big change observed from graphene to TBG is very intriguing but unclear, because it is very counterintuitive to ascribe such a big change to the tiny change in twist or to the very weak van der Waals force (vdW) interlayer interaction.To comprehend the huge difference due to tiny change in TBG, we examined the electronic properties of graphene and conventional bilayer graphene, created twisted bilayer graphene and investigated the electronic band structure of TBG within tight binding approximation and effective continuum model. The electrons move extremely slowly in the flat band near the Fermi level, increasing the Coulomb interaction between each other, or the so-called strong correlation effect, which can help us understand the emergence of superconductivity relevant to high-Tc superconductors(Cao, Fatemi, Demir, Fang, Tomarken, Luo, Sanchez-Yamagishi, Watanabe, Taniguchi, Kaxiras, Ashoori, & Jarillo-Herrero, 2018; Cao, Fatemi, Fang, Watanabe, Taniguchi, Kaxiras, & Jarillo-Herrero, 2018)

Atomic and Electronic Structure of Monolayer Graphene
Atomic and Electronic Structure of Bilayer Graphene
Atomic Structure and Electronic Band of Twisted Bilayer Graphene
The Effective Continuum Model and Electronic Band of TBG
Discussion
Conclusion
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