Abstract
The three-dimensional Eulerian model CAMx (Comprehensive Air QualityModel with Extensions) was applied for the first time to simulate bothgaseous and particulate photochemical air pollution in Switzerland during July 28–30, 1993. The meteorological input data were prepared using the Systems Applications International Mesoscale Model (SAIMM). The CAMx model results were compared with the measurements carried out at ground level andfrom airborne measuring platforms within the frame of the Swiss POLLUMET research programme. In general, the CAMx performance for gaseous species wasfound to be better than that of the previously used Urban Airshed Model (UAM)and the Variable Grid Urban Airshed Model (UAM-V). The most significant improvement for the gaseous species is in the prediction of HNO3 concentrations, due to the inclusion of aerosol chemistry. Aerosol species such as NO3 -, NH4 +, SO4 2-, and secondary organic aerosols were calculated in one particle size range (0.04–2.5 μm) and compared with a few measurements available. Although July 29 was reasonably well simulated, overestimated wind speeds by SAIMM for July 30 caused a too fast transport of pollutants. Similarly to measurements, significant spatial correlation of the secondarily formed aerosols with ozone and formaldehyde is found in the afternoon.
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