Abstract

Due to the rapid economic growth and the heavy reliance on fossil fuels, China has become one of the countries with the highest sulfur dioxide (SO2) emissions, which pose a severe challenge to human health and the sustainable development of social economy. In order to cope with the serious problem of SO2 pollution, this study attempts to explore the spatial temporal variations of industrial SO2 emissions in China utilizing the Defense Meteorological Satellite Program’s Operational Linescan System (DMSP-OLS) nighttime stable light (NSL) data. We first explored the relationship between the NSL data and the statistical industrial SO2 emissions at the provincial level, and confirmed that there was a positive correlation between these two datasets. Consequently, 17 linear regression models were established based on the NSL data and the provincial statistical emissions to model the spatial-temporal dynamics of China’s industrial SO2 emissions from 1997 to 2013. Next, the NSL-based estimated results were evaluated utilizing the prefectural statistical industrial SO2 emissions and emission inventory data, respectively. Finally, the distribution of China’s industrial SO2 emissions at 1 km spatial resolution were estimated, and the temporal and spatial dynamics were explored from multiple scales (national scale, regional scale and scale of urban agglomeration). The results show that: (1) The NSL data can be successfully applied to estimate the dynamic changes of China’s industrial SO2 emissions. The coefficient of determination (R2) values of the NSL-based estimation results in most years were greater than 0.6, and the relative error (RE) values were less than 10%, when validated by the prefectural statistical SO2 emissions. Moreover, compared with the inventory emissions, the adjusted coefficient of determination (Adj.R-Square) reached 0.61, with the significance at the 0.001 level. (2) During the observation period, the temporal and spatial dynamics of industrial SO2 emissions varied greatly in different regions. The high growth type was largely distributed in China’s Western region, Central region, and Shandong Peninsula, while the no-obvious-growth type was concentrated in Western region, Beijing-Tianjin-Tangshan and Middle south of Liaoning. The high grade of industrial SO2 emissions was mostly concentrated in China’s Eastern region, Western region, Shanghai-Nanjing-Hangzhou and Shandong Peninsula, while the low grade mainly concentrated in China’s Western region, Middle south of Liaoning and Beijing-Tianjin-Tangshan. These results of our research can not only enhance the understanding of the spatial-temporal dynamics of industrial SO2 emissions in China, but also offer some scientific references for formulating feasible industrial SO2 emission reduction policies.

Highlights

  • Sulfur dioxide (SO2) is one of the main pollutants in the atmosphere, which is an important indicator to measure whether the atmosphere is polluted [1]

  • In order to cope with the industrial SO2 pollution problems in China, this study explored the spatiotemporal dynamics of industrial SO2 emissions from 1997 to 2013, and put forward relevant suggestions on industrial SO2 emission mitigation

  • On the basis of proving that there was a positive correlation between the DMSP-OLS stable lights and industrial SO2 emissions, we tried to utilize nighttime stable light (NSL) data to simulate industrial SO2 emissions

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Summary

Introduction

Sulfur dioxide (SO2) is one of the main pollutants in the atmosphere, which is an important indicator to measure whether the atmosphere is polluted [1]. SO2 is released when burning materials containing sulfur, which is found in all types of coal and oil across the world in varying proportions. SO2 in the atmosphere can be emitted from both natural and anthropogenic sources [7]. Natural SO2 sources mainly come from oxidation of biogenic dimethyl sulfide and volcanic eruption [8]. The primary anthropogenic SO2 emission is from fossil fuel consumption, especially for power generation, and other industrial production activities [9]. It is estimated that anthropogenic emissions are the main source of global SO2 emissions [10, 11]

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