Abstract
AbstractMonte Carlo simulation was used to model the fractionation process in crystallization analysis fractionation (CRYSTAF). Five poly(ethylene/1‐octene) samples synthesized with a single‐site–type catalyst were used to verify the simulation results. It was proposed that the fractionation mechanism be controlled by the crystallization of the longest ethylene sequence in each chain. Good agreement between experimental and simulation results verified the validity of the proposed fractionation mechanism. © 2001 John Wiley & Sons, Inc. J Appl Polym Sci 80: 2200–2206, 2001
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