Abstract
) is the ideal spin center for MCEas it has a high isotropic spin; however, the internal natureof the 4f electrons hampers the magnetic communicationbetween them. A mixed-metal 3d–4f approach should havethe advantage of a better magnetic interaction and thus,a larger ground spin in the preferred ferromagnetic case. Wehave used this approach to make cobalt(II) (s=3/2) andnickel(II) (s=1) gadolinium phosphonate complexes withlarge MCEs.
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