Abstract
The structural and magnetic behavior of Mn-site doped intermetallic manganese silicide alloys of nominal compositions Mn5−xAxSi3 (x = 0.05, 0.1, 0.2 and A = Ni, Cr) have been investigated with a focus to the inverted hysteresis behavior and thermomagnetic irreversibility. Room temperature x-ray powder diffraction data confirm that all the doped alloys crystallize in hexagonal D88 type structure with space group P63/mcm. The doped alloys are found to show paramagnetic–collinear antiferromagnetic (AFM2)–noncollinear antiferromagnetic (AFM1) transitions during cooling from room temperature. A significant decrease in the critical values of both AFM1–AFM2 transition temperatures and fields have been observed with the increasing Ni/Cr concentration. Inverted hysteresis loop, field-induced arrest, and thermomagnetic arrest, the key features of the undoped Mn5Si3 alloy, are found to be significantly affected by the Mn-site doping and eventually vanishes with 4% doping.
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