Abstract

Abstract. The MIX inventory is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) by a mosaic of up-to-date regional emission inventories. Emissions are estimated for all major anthropogenic sources in 29 countries and regions in Asia. We conducted detailed comparisons of different regional emission inventories and incorporated the best available ones for each region into the mosaic inventory at a uniform spatial and temporal resolution. Emissions are aggregated to five anthropogenic sectors: power, industry, residential, transportation, and agriculture. We estimate the total Asian emissions of 10 species in 2010 as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.6 Tg CO, 67.0 Tg NMVOC (non-methane volatile organic compounds), 28.8 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2. Emissions from China and India dominate the emissions of Asia for most of the species. We also estimated Asian emissions in 2006 using the same methodology of MIX. The relative change rates of Asian emissions for the period of 2006–2010 are estimated as follows: −8.1 % for SO2, +19.2 % for NOx, +3.9 % for CO, +15.5 % for NMVOC, +1.7 % for NH3, −3.4 % for PM10, −1.6 % for PM2.5, +5.5 % for BC, +1.8 % for OC, and +19.9 % for CO2. Model-ready speciated NMVOC emissions for SAPRC-99 and CB05 mechanisms were developed following a profile-assignment approach. Monthly gridded emissions at a spatial resolution of 0.25° × 0.25° are developed and can be accessed from http://www.meicmodel.org/dataset-mix.

Highlights

  • The Model Inter-Comparison Study for Asia (MICS-Asia) project is currently in phase III

  • A reasonable understanding of anthropogenic emissions is essential for atmospheric chemistry and climate research (Xing et al, 2013; Keller et al, 2014)

  • The industrial sector has the largest contribution to SO2 (50 % of total), NMVOC (38 %), PM10 (48 %), and CO2 (40 %) emissions

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Summary

Introduction

The Model Inter-Comparison Study for Asia (MICS-Asia) project is currently in phase III. During the previous two phases, studies have been focused on long-range transport and deposition of pollutants, global inflow of pollutants to Asia, model sensitivities to aerosol parameterization, and emissions over Asia (Carmichael et al, 2002, 2008; Han et al, 2008; Hayami et al, 2008; Holloway et al, 2008; Wang et al, 2008). MICS-Asia Phase III aims to conduct further intercomparisons of atmospheric modeling for Asia and analyze the disagreement of model output and relative uncertainties. In this regard, common meteorological fields, emission data, and boundary conditions should be used. One of the key tasks in MICS-Asia Phase III is to develop a reliable Asian emission inventory as common input for model intercomparisons through integration of state-of-the-art knowledge on Asian emissions. For a large geographic region like Asia, compiling a bottom-up emission inventory is a challenging task because it requires a huge amount of local information on energy use, technologies, and environmental regulations for many different countries

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