Abstract

In the past decade, mid-infrared (MIR) few-cycle lasers have attracted remarkable research efforts for their applications in strong-field physics, MIR spectroscopy, and bio-medical research. Here we present a review of MIR few-cycle pulse generation and amplification in the wavelength range spanning from 2 to ~20 μm. In the first section, a brief introduction on the importance of MIR ultrafast lasers and the corresponding methods of MIR few-cycle pulse generation is provided. In the second section, different nonlinear crystals including emerging non-oxide crystals, such as CdSiP2, ZnGeP2, GaSe, LiGaS2, and BaGa4Se7, as well as new periodically poled crystals such as OP-GaAs and OP-GaP are reviewed. Subsequently, in the third section, the various techniques for MIR few-cycle pulse generation and amplification including optical parametric amplification, optical parametric chirped-pulse amplification, and intra-pulse difference-frequency generation with all sorts of designs, pumped by miscellaneous lasers, and with various MIR output specifications in terms of pulse energy, average power, and pulse width are reviewed. In addition, high-energy MIR single-cycle pulses are ideal tools for isolated attosecond pulse generation, electron dynamic investigation, and tunneling ionization harness. Thus, in the fourth section, examples of state-of-the-art work in the field of MIR single-cycle pulse generation are reviewed and discussed. In the last section, prospects for MIR few-cycle lasers in strong-field physics, high-fidelity molecule detection, and cold tissue ablation applications are provided.

Highlights

  • The mid-infrared (MIR) wavelength is usually defined in the range of 2–20 μm (500–5000 cm−1 )

  • We review typical MIR nonlinear crystals and summarize the techniques for the generation and amplification of ultrafast MIR lasers, including optical parametric amplification (OPA), optical parametric chirped-pulse amplification (OPCPA), and intrapulse difference-frequency generation (IPDFG) with various kinds of designs

  • Nonlinear crystals that are commonly used in MIR pulse generation and amplification mainly include KTiOAsO4 (KTA), KTiOPO4 (KTP), and LiNbO3 (LNO), which belong a group known as oxide crystals, and ZnGeP2 (ZGP), CdSiP2 (CSP), AgGaS2 (AGS), AgGaSe2 (AGSe), GaSe, BaGa4 S7 (BGS), BaGa4 Se7 (BGSe), LiGaS2 (LGS), and LiGaSe2 (LGSe), which are classified as non-oxide crystals

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Summary

Introduction

The mid-infrared (MIR) wavelength is usually defined in the range of 2–20 μm (500–5000 cm−1 ). As for MIR solid-state lasers, there are two main technique streams to generate MIR pulses, namely the direct emission of doped ions and optical parametric down conversion. The former is based on a process wherein the gain medium is stimulated after energy storage, and the output wavelength depends on the energy level structures of the gain media. The second technique is based on the parametric frequency conversion that is mainly assisted by nonlinear crystals that create the phase-matching conditions In this process, there is no thermal accumulation, and broadband laser amplification can be realized through broadband phase matching, which supports the generation of few-cycle MIR pulses. New prospects for MIR few-cycle lasers in strong-field physics, high-fidelity molecule detection, and cold tissue ablation applications are provided

MIR Nonlinear Crystals
MIR Generation
Experimental setup setup of of MIR
MIR OPCPA
Illustration
Schematic
Layout
10. Schematic
12. Setup ofofthe
MIR Intra-Pulse DFG
17. Schematic forfor
Single-Cycle
MIR Single-Cycle Pulse Generation via DFG
MIR Single-Cycle Pulse Generation via FWM
MIR Single-Cycle Pulse Generation via IPDFG
Prospects of High-Power Broad-Band Few-Cycle MIR Lasers
Findings
Conclusions

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