Abstract

Microwave-absorbing materials (MAMs) are essential for mitigating the unwanted effects of electromagnetic interference and microwave pollution. MAMs are also used in 5G technology, energy harvesting, information security, and military technology (such as reduced radar cross-section). In this work, SrFe12–2xCux/2Cox/2TixO19 samples, prepared by using a ball mill and heat treatment method, showed their superior microwave dissipation features in both effective absorption bandwidth (EAB) and reflection loss (RL) values for the microwave incident angle of 0°, where EAB and RL values reached 15.90 GHz and −42.86 dB, respectively. The optimum RL values would change with the variation of the incident microwave angle. RL values at a specific oblique angle could exhibit better RL values for both transverse electric (TE) and transverse magnetic (TM) polarization modes, except for the x = 0.15 (SrM15) sample for TE mode. In detail, the x = 0 (SrM0) sample achieved the lowest RL value of −71.28 dB for the incident angle of 20° in the TE polarization mode, which was much better than that of the normal incident. The RL of the SrM15 sample in TM mode was significantly enhanced and reached a value of −66.48 dB for an incident angle of 10°. The increase in the RL values resulted from the superior values of complex permittivity and permeability and their matching. In addition, the improvement in RL values could be attributed to the increase in incident and refraction angles as well as the longer pathway of the microwave inside the samples. These discoveries also illustrate that SrFe12–2xCux/2Cox/2TixO19 samples hold promise for various everyday applications, even when exposed to oblique angle variation.

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