Abstract

AbstractOptical pumping conditions for organic solid‐state lasers (OSLs) are discussed with particular emphasis on the use of gallium nitride based light‐emitting diodes (LEDs) as pump sources. LEDs operate in a regime where the pump should be optimized for a short rise time and high peak intensity, whereas fall time and overall pulse duration are less important. Lasers pumped with this approach need to have very low thresholds which can now be routinely created using (one‐dimensional) distributed feedback lasers. In this particular case stripe‐shaped excitation with linearly polarized light is beneficial. Arrays of micron‐sized flip‐chip LEDs have been arranged in an appropriate stripe shape and the array dimensions were chosen such that the divergence of LED emission does not cause a loss in peak intensity. These micro‐LED arrays have successfully been used to pump OSLs with thresholds near 300 W/cm2 (∼9 ns rise time, 35 ns pulse duration), paving the way for compact arrays of indirectly electrically pumped OSLs.

Highlights

  • Organic chromophores have always played an important role in photonics

  • Various aspects of optical pumping conditions of organic solid-state lasers (OSLs) have been discussed with particular emphasis on using GaN light-emitting diodes (LEDs) as pump sources

  • Simulation results show that the pump pulse duration and the pulse shape and in particular its rise time have a strong influence on the laser threshold

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Summary

Introduction

Organic chromophores have always played an important role in photonics. Considerable efforts are undertaken to exploit them for solid-state laser sources because they offer simple fabrication methods and access to the whole visible spectrum (including schemes for mechanical and electrical laser wavelength tuning) as well as potential for mechanically flexible devices. This article will concentrate on optical pumping and in particular the use of GaN light-emitting diodes (LEDs) as pump sources Such an approach aims to make a virtue of optical pumping and enable compact devices which closely mimic the properties a directly electrically driven device would have. We present the systematic improvement of organic lasers and pumping conditions with the particular objective to use arrays of micron-sized flip-chip GaN LEDs [15, 16] as pump source. This LED format was chosen because it holds potential for enhanced functionality in future devices such as pattern programmability and potential for integration with CMOS control electronics [16]. This effort led to the demonstration of an OSL pumped by micro-LEDs

Gain Dynamics in Organic Gain Media
Relevant Parameters
Details of the Model
Towards CW OSLs
Optical Gain under Pulsed Pumping
Different Regimes of OSL Pumping
Implications for LED and LD pumping
Flip-Chip Micro-LEDs for OSL Pumping
Pump Setup
Actual Pump Spot Dimensions
Pulsed Operation
Limitation of LED Pulsed Output
Micro-LED Performance
Summary of micro-LED Performance
Laser Thresholds
Organic Lasers for Integration with LEDs
Outstandingly low thresholds
Material Choice
Pump Spot Geometry and Pump Polarization
Low-threshold OSLs for LED Pumping
Findings
Conclusion

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