Methodologies to obtain aerosol property profiles from three-wavelength elastic lidar signals

Abstract

The Lidar/Radiometer Inversion Code (LIRIC) and the Constrained Iterative Inversion (CII) procedure combined with a graphical aerosol classification framework (GF) have been used to analyse their ability in characterizing the altitude dependence of aerosol properties and evaluate their benefits and weaknesses. LIRIC and the CII technique rely on elastic lidar signals at 355, 532, and 1064 nm and collocated Aerosol Robotic Network (AERONET) Sun/sky photometer measurements to retrieve aerosol parameter profiles at the lidar wavelengths. The aerosol GF relies on the combined analysis of the Ångström exponent at the wavelength pairs 355 and 1064 nm (A(355, 1064)) and its spectral curvature (ΔA = A(355, 532) – A(532, 1064)) to estimate the fine-modal radius and the 532 nm fine-mode fraction. The application of the LIRIC and CII-GF techniques to three selected case studies representative of Central Mediterranean aerosol scenarios has revealed that the differences between the aerosol products from LIRIC and the corresponding ones from the CII-GF procedure varied with altitude, increased with the lidar wavelength decrease, and were significantly large when aerosol from different sources and/or from different advection routes was located at the altitudes sounded by the lidar. The plot on the aerosol GF of A(355, 1064) versus the spectral curvature has indicated that the LIRIC constraint that the fine-modal radius is height independent may represent a weakness if aerosol types and hence aerosol size distributions vary with altitude. The use of lidar ratios (LRs) constant with altitude could represent one of the main weaknesses of the CII-GF technique. The combined use of both techniques should allow obtaining a better characterization of the altitude dependence of aerosol properties from three-wavelength elastic lidar signals.