Abstract
AbstractAn efficient method for the direct construction of pyrimidines from a metal‐free, TBHP‐mediated, [3+2+1]‐type intermolecular cycloaddition reaction from amidines, ketones, and DMF through C(sp3)−H activation has been developed. This transformation involves the formation of new C−C/C−N bonds and features sustainable oxidants, readily available starting materials, and high atom and step economies.
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