Abstract
We successfully synthesized mesocrystalline Ta2O5 nanosheets supported bimetallic PdPt nanoparticles by the photo-reduction method. The as-prepared mesocrystalline Ta2O5 nanosheets in this work showed amazing visible-light absorption, mainly because of the formation of oxygen vacancy defects. And the as-prepared bimetallic PdPt/mesocrystalline Ta2O5 nanaosheets also showed highly enhanced UV–Vis light absorption and highly improved photocatalytic activity for hydrogen production in comparison to that of commercial Ta2O5, mesocrystalline Ta2O5 nanosheets, Pd/mesocrystalline Ta2O5 nanosheets and Pt/mesocrystalline Ta2O5 nanosheets. The highest photocatalytic hydrogen production rate of PdPt/mesocrystalline Ta2O5 nanaosheets was 21529.52 g−1 h−1, which was about 21.2 times of commercial Ta2O5, and the apparent quantum efficiency of PdPt/mesocrystalline Ta2O5 nanaosheets for hydrogen production was about 16.5% at 254 nm. The highly enhanced photocatalytic activity was mainly because of the significant roles of PdPt nanoparticles for accelerating the charge separation and transport upon illumination. The as-prepared PdPt/mesocrystalline Ta2O5 nanaosheets in this work could serve as an efficient photocatalyst for green energy production.
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