Abstract
To probe the reactivity of ionic liquids relevant to their use in electrochemical applications, the ionic liquid 1-ethyl-3-methylimidazolium tetrachloroaluminate(III) was reacted with metallic lithium to produce a persistent radical, which can be considered a hydrogen-atom adduct of an electron-rich olefin (ERO). Reaction of tetrakis(dimethylamino)ethene, a bona fide ERO, with muonium, produces a structurally similar radical.
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