Abstract
The ionic SN2-type mechanistic pathway initiated by silane end-on coordination on the metal centers, forming η1-H(Si) Mo/W complexes, is the preferred reaction pathway for the two cationic cyclopentadienyl molybdenum/tungsten complexes, [CpM(CO)2(IMes)]+ (M = Mo, W) in catalyzing carbonyl hydrosilylation.
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