Abstract

The ionization of bicyclo[1.1.1]pentyl-1 derivatives is shown to involve rearrangement to the bicyclo[1.1.0]butyl-1-carbinyl cation rather than the 3-methylenecyclobutyl cation. This is in good accord with MP2-6-31G * theoretical predictions and is in contrast to the products of solvolysis which are 3-methylenecyclobutyl derivatives

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