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Abstract
Alkali-activated slag (AAS) binders-based composites are considered potential alternatives to conventional cement-based composites. However, the quasi-brittle mechanical behavior of AAS binders-based composites limits their widespread application. In this study, a graphene oxide-SiO2 (GO-SiO2) composite was produced to address this issue. The experimental results showed that the flexural strength of an AAS paste increased by 133.2% with 1.5 wt% GO-SiO2 composite, and its corresponding flexural-to-compressive strength ratio increased 95% i.e. from 0.063 to 0.123. To explore the strengthening mechanism, the stability of the GO-SiO2 composite in alkaline solutions and the dispersion effect of GO-SiO2 composite on the mechanical properties of AAS paste were investigated. The experimental results showed that the prepared GO-SiO2 composite had stable C–O–Si chemical bonds connected GO with hydration products, thereby improving the strength of the AAS paste. The molecular dynamics study revealed the mechanism that the high-dispersed GO-SiO2 composite could improve the mechanical properties of the AAS paste dramatically.
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