Abstract

Abstract. In this paper, we present measurements of total and tropospheric ozone, retrieved from infrared radiance spectra recorded by the Infrared Atmospheric Sounding Interferometer (IASI), which was launched on board the MetOp-A European satellite in October 2006. We compare IASI total ozone columns to Global Ozone Monitoring Experiment-2 (GOME-2) observations and ground-based measurements from the Dobson and Brewer network for one full year of observations (2008). The IASI total ozone columns are shown to be in good agreement with both GOME-2 and ground-based data, with correlation coefficients of about 0.9 and 0.85, respectively. On average, IASI ozone retrievals exhibit a positive bias of about 9 DU (3.3%) compared to both GOME-2 and ground-based measurements. In addition to total ozone columns, the good spectral resolution of IASI enables the retrieval of tropospheric ozone concentrations. Comparisons of IASI tropospheric columns to 490 collocated ozone soundings available from several stations around the globe have been performed for the period of June 2007–August 2008. IASI tropospheric ozone columns compare well with sonde observations, with correlation coefficients of 0.95 and 0.77 for the [surface–6 km] and [surface–12 km] partial columns, respectively. IASI retrievals tend to overestimate the tropospheric ozone columns in comparison with ozonesonde measurements. Positive average biases of 0.15 DU (1.2%) and 3 DU (11%) are found for the [surface–6 km] and for the [surface–12 km] partial columns respectively.

Highlights

  • Global monitoring of ozone (O3) is essential since this molecule plays a key role in the photo-chemical equilibrium of the atmosphere

  • Retrievals are only performed for cloud-free scenes, identified using a filter based on the estimation of brightness temperatures around 11 and 12 μm and on their comparison with the surface temperature provided by the European Centre for Medium-Range Weather Forecasts (ECMWF) analyses

  • Retrievals of total and tropospheric ozone columns from radiances measured by the Infrared Atmospheric Sounding Interferometer (IASI) instrument have been performed

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Summary

Introduction

Global monitoring of ozone (O3) is essential since this molecule plays a key role in the photo-chemical equilibrium of the atmosphere. Ozone is one of the main greenhouse gases and plays a major role in determining the oxidizing capacity of the troposphere. For all these reasons, ozone needs to be monitored with good spatial and temporal coverage in order to better understand its evolution and its impact on air quality and climate. There are currently three nadir viewing TIR instruments providing ozone measurements from polar-orbiting satellites: the Atmospheric InfraRed Sounder (AIRS) on AQUA, the Tropospheric Emission Spectrometer (TES) on AURA and the Infrared Atmospheric Sounding Interferometer (IASI) on MetOp-A. 3, the IASI total and tropospheric ozone columns are compared with correlative ozone measurements, obtained by the GOME-2 instrument on board the MetOp-A platform, ground-based and ozonesonde data.

IASI data
Ozone retrievals
Total ozone global distributions
Ozone vertical profiles
Comparisons with GOME-2 measurements
Comparisons with ground-based measurements
Tropospheric ozone
Findings
Summary and conclusions
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