Measurements of neutron capture cross-sections for 187Re isotope around 14 MeV neutrons and theoretical calculations of excitation functions

Abstract

The cross-sections of the 187Re(n,γ)188mRe and 187Re(n,γ)188gRe reactions were measured at the four neutron energies of 13.5, 14.1, 14.4 and 14.8 MeV through the activation method and using off-line γ-ray spectrometry. The previously developed formulas were used to subtract the effects of γ rays with close energies and the contribution from the excited state. A high-resolution γ-ray spectrometer with high-purity germanium detector was used to measure the induced γ activities. The simulation computations of the excitation functions concerning the above-mentioned two nuclear reactions were performed by adopting the nuclear theoretical model program system Talys-1.9. The theoretical excitation curves in the incident neutron energy range from 2.53 × 10−8 to 20 MeV were acquired. The fitting line of our results in the neutron energy range of 13.5–14.8 MeV, within experimental uncertainty, agrees very well with the theoretical excitation curve based on the computer code Talys-1.9.