Measurements of excitation functions of α-particle induced reactions on natNi: possibility of production of the medical isotopes 61Cu and 67Cu

Abstract

Abstract Excitation functions of the natNi(α,x)60,61Cu and 64Ni(α,p)67Cu reactions were measured using the stacked-foil activation technique. The experimental data achieved were compared with literature data as well as with nuclear model calculations performed using the code TALYS-1.8. Integral yields from the respective thresholds to 44 MeV were deduced from the measured excitation curves. The >99% pure 61Cu can be produced using the energy window of Eα=20→7 MeV, the yield amounting to 116 MBq/μAh. After a 2 h cooling time, the short-lived 60Cu (T1/2=23 min) impurity will be reduced to <0.1%. Due to low isotopic abundance of 64Ni, the enriched 64Ni target would be needed for the production of 67Cu via the (α,p) reaction. The cost would, however, be very high. In a few cases, particularly above 24 MeV, we have given new data points. In general, our measurements have strengthened the database.