Measurement of the (n, 2n) reaction cross-sections of iodine and cesium induced by D-T neutrons with covariance analysis* *Supported by the Key Laboratory of Nuclear Data Foundation (JCKY2022201C151), and the National Natural Science Foundation of China (11975113).

Abstract

The cross-sections of the 127I (n, 2n) 126I and 133Cs (n, 2n) 132Cs reactions at neutron energies of 13.83 ± 0.05, 14.33 ± 0.10, and 14.79 ± 0.10 MeV were measured relative to the 93Nb (n, 2n) 92mNb reaction using the activation technique in combination with off-line γ-ray spectrometry. A neutron beam was generated from the T (d, n) 4He reaction using the K-400 neutron generator at the China Academy of Engineering Physics. Considering the correlations between different attributes, detailed uncertainty propagation was performed using covariance analysis, and the cross-sections were reported with their uncertainties and correlation matrix. The uncertainty of the measurement cross-sections ranged from 4.84 to 5.90%, which is lower than previous experimental data. Furthermore, the theoretical excitation functions of the 127I (n, 2n) 126I and 133Cs (n, 2n) 132Cs reactions were calculated using the TALYS-1.95 and EMPIRE-3.2.3 codes. Then, the experimentally determined cross-sections were analyzed by comparing them with literature data available in the EXFOR database and evaluated nuclear data in the ENDF/B-VIII.0, JEFF-3.3, JENDL-5, BROND-3.1, CENDL-3.2, and TENDL-2021 databases. Compared with the values previously reported in the 13.8-14.8 MeV energy region, the precision of the results obtained in this study was greatly improved. The current experimental results with thorough uncertainties and covariance information are critical for verifying the reliability of the theoretical model and improving the quality of the nuclear database.