Abstract
The three independent second-order nonlinear optical coefficients of BaMgF4 are determined by the Maker fringe method with a nanosecond pulsed Nd:YAG laser at 1064 nm wavelength. All the results are relative to the reference crystal congruent LiNbO3. The largest element in a second-order nonlinear optical matrix of BaMgF4 is d32, with the value of 0.36 pm/V.
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