Measurement of 232Th(n,f) and 232Th(n,γ) reaction rates in thorium powder cylinder bombarded with D-T neutrons

Abstract

ABSTRACTIn order to provide reference for the evaluation of thorium parameters for the conceptual design of fusion–fission hybrid energy reactor, a dedicated integral experiment was carried out in a thorium powder cylinder bombarded with D-T neutrons. Thorium capture and fission rates in the 0° direction to the incident D+ beam were obtained using the activation method followed by the off-line gamma-ray technique, experimental uncertainties were ∼3.1% for thorium capture rate, and were 5.5%, 8.1%, and 6.3% for thorium fission rates based on fission products 85mKr, 143Ce, and 87Kr, respectively. The thorium fission rate based on 85mKr agreed well with the simulation employing ENDF/B-VII.0 library data. The influence of the oxygen contained in the thorium oxide powder and the scattering neutrons from the experimental hall was also evaluated. MCNP simulations employing ENDF/B-Ⅶ.0, JENDL-4.0 library data agreed with experiment within uncertainties except that employing ENDF/B-Ⅶ.1 (6.0%) and CENDL-3.1 (7.9%) for thorium fission rate, while for thorium capture rate, simulation employing JENDL-4.0 agreed with experiment best. The influence of reaction channels of thorium transport medium employing different library data on the thorium reaction rates could be neglected according to the simulation. The thorium capture to fission ratio demonstrated that the fuel breeding efficiency is quite low and energy production plays a leading role under the neutron spectra in this experiment.