Measurement and calculations of long-lived radionuclide activity forming in the fast neutron field in some ITER construction steels

Abstract

Measurement and calculations of long-lived gamma-emitting radionuclide activity forming in the fission reactor fast neutron field were done, for some ITER construction steels. The activation was conducted in fast neutron irradiation channel of the MARIA research fission reactor (Poland). The dimensions of steel samples were 10mm×10mm×1mm and mass was approximately 0.8g. The neutron flux density was measured by means of activation foil method and unfolding technique; fraction of neutrons above 1keV was 95%. The activation lasted 242h and cooling took 100 days; the mean neutron flux density was 2.9E12 n/(cm2s) (neutrons above 500keV are 53% of total) whereas total fluency 2.53E18cm−2. The activity measurements were done by means of gamma-ray spectrometry. Activity calculations were done by means of FISPACT-II code using the activation libraries EAF-2010 and TENDL-2011 and experimentally determined neutron flux. Measured activity of long-lived gamma emitting radionuclides was, in average, about 6.3MBq/g 100 days after activation; the dominant radionuclides were 58Co and 54Mn (about 81% and 14% of total activity respectively). The C/E ratio differs for particular radionuclides and is in the range 0.86–0.92 for 51Cr, 0.93–1.21 for 54Mn, 0.77–0.98 for 57Co, 0.91–1.21 for 58Co, 1.17–1.27 for 59Fe, and 1.75–2.44 for 60Co.