Abstract
The hybridization in cyclobutane, bicyclobutane, 1,3-dimethylcyclobutane, 1,3-dimethylbioyclobutane, bicyclo(1.1.1)pentane, tricyclo(1.1.0.02,4)butane, cubane and tetracyclo-(3.3.1.02,804,6)nonane is considered applying the method of maximum overlap (Tab. 1). Overlap seems to be a good index of a CC bond: overlaps below 0.6000 are characteristic for molecules containing C3-ring (δ ∼ 20‡), between 0.6000 and 0.6300 for four membered ring (δ ∼ 10‡), and above 0.6300 for normal or very slightly bent bonds (δ<5‡). Description and details of actual numerical calculations are given.
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