Abstract

The geochemical characteristics of mantle degassing observed on the surface of the earth can indicate the origin and migration path of mantle fluids. Compared with the plate boundary tectonic environment, the intraplate tectonic environment does not have a large number of active volcanoes and active faults, and the observation of mantle volatiles in hot spring gas is relatively limited. We selected the Sichuan–Yunnan block to discuss mantle degassing based on the carbon and noble gas isotopes of the spring gases and previous studies on the fault slip rate and geophysical research. A total of five hot spring gas samples (including two free gases and three dissolved gases) were collected from the Sichuan–Yunnan block. Chemical and isotopic compositions were analyzed in N2-dominant hot spring gases. The 3He/4He ratio (0.068–0.541 Ra) indicates the occurrence of mantle-derived helium throughout the Sichuan–Yunnan block, which has been diluted by a crustal radiogenic 4He component. The occurrence of mantle-derived helium in the study areas ranges from 0.74 to 5.67%. The lower proportion of mantle-derived helium in YNWQ and HGWQ than that in other spring gases near the Jinghe-Qinghe fault may be caused by the smaller scale of fault around YNWQ and HGWQ than the Jinghe-Qinghe fault. The correlation between 4He, 20Ne, and N2 concentrations implies a common trapping mechanism for 4He, 20Ne, and N2 in hot spring gases. The 40Ar/36Ar ratios and N2/Ar ratios indicate that N2 and Ar are mostly meteoric, and YNWQ and HGWQ have more crustal-derived Ar contribution (40.56 and 51.49%, respectively). The δ13C(CO2)o values calculated by Rayleigh fractionation and CO2 concentration suggest that CO2 has inorganic and organic origins. The plot of Rc/Ra versus δ13C(CO2) indicates that the spring gas CO2 origin in the Sichuan–Yunnan block is mainly derived from mixing of limestone and organic sediments with minor mantle CO2. The δ13C(CH4) versus CH4/3He values indicate that the origin of methane is thermogenic and microbial oxidation. The low mantle-derived helium distribution pattern is most likely controlled by the weak fault activity rate, the small fault scale, and not obvious magmatic activity in the Sichuan–Yunnan block.

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