Abstract
The absorption band profiles of the magnon sideband associated with lowest energy component of 6A1g→4T1g(D) have been measured in two-dimensional antiferromagnets (RNH3)2MnCl4(R = Me, Et, Prn, PhCH2) to correlate the bandshape with the extent of puckering in the Mn–Cl layers; no simple correlation exists with any single crystallographic parameter.
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