Abstract
Ba0.8Sr0.2TiO3–CoFe2O4 (BST–CFO) multilayered composite films were prepared on Pt/Ti/SiO2/Si substrates via a sol–gel method and spin-coating technique. Microstructures, electric property, magnetic property and magnetoelectric (ME) property of the composites were studied. Results show that the composite films calcined at 750 °C have BST and CFO phases and no obvious impurity phases were detected. Further, the composite films exhibit layered structures and a transition layer which is composed of interfacial delamination exists at the interface between BST and CFO layers. Ferroelectric and ferromagnetic properties were simultaneously observed in the films, evidencing the coexistence of the ferroelectric and ferromagnetic properties. Furthermore, the saturation magnetization value of the composite film is lower than that of the pure CFO film derived by the same processing as a result of the effect of the nonferromagnetic BST layers. Also, ferroelectric hysteresis loops reveal that the saturated polarization and remanent polarization of the composite film are lower than those of the pure BST films. In addition, the composite film exhibits a strong ME effect, which makes the composite film attractive for technological applications as devices.
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