Magneto-optical properties of bilayer phosphorene quantum dots.

Abstract

Using the tight-binding approach, we investigate the electronic and magneto-optical properties of bilayer phosphorene quantum dots (BLPQDs) in the presence of perpendicular electric and magnetic fields. The magneto-energy spectra of the BLPQDs exhibit Aharonov-Bohm oscillations. The period and the amplitude of the oscillation decrease with the size of the BLPQDs. An oscillatory behavior of the local density of states (LDOS) versus the magnetic field is observed, as well as the appearance of the spatial Aharonov-Bohm oscillations in the LDOS. In the absence of the electric field, there exists an s-fold degeneracy (s absolutely flat bands at exactly zero energy) arising from the edge-mode states, where s is the smaller value between M and N, where M and N are the number of phosphorus atoms along the x and y axis, respectively, in a rectangular BLBPQD. The absorption spectra of the BLPQDs are obtained for both in-plane and out-of-plane polarizations. Compared with the absorption spectra of graphene dots, the absorption of an out-of-plane polarization of the incident light is high compared to that of in-plane polarizations. On the other hand, the absorption spectra due to in-plane polarizations are almost the same in the case of graphene, whereas they are considerably different in BLBPQDs. Importantly, the appearance of several sharp and high absorption peaks in the near-infrared (NIR) range dictates the BLBPQDs for application and development of bioimaging, biomedicine and drug delivery technology. More importantly, both the location and intensity of these NIR peaks depend characteristically on the orientation of the polarization of the incident light, which can be desirably tuned by the simultaneous engineering of magnetic and electric fields. Such unique advantage of the anisotropic optical feature enables a new degree of freedom for achieving novel polarization-dependent photonic devices. The dual magnetic and electric field tunable optical and electrical features of the BLPQDs are expected to have important consequences for the development of multifunctional magneto-optoelectronic devices and provide insight into the applicability of quantum photopic technologies based on BLBPQDs.