Abstract
Charge transfer (CT) complexes are promising for developing molecule-based magnets, where ~ -electrons play an important role. New classes of molecular magnets are presented in the TTF-based CT complexes from points of unconventional magnetism. ~ -d interaction in d-electron-spin-incorporated CT complexes give anomalous effect of magnetic transition on the electron transport. The coexistence of metallic conduction and localized spin feature appears in the system located in the metal-insulator boundary. 1D metal having ferromagnetic interaction and triangle-based spin ladder system are also obtained from CT complexes. organic metal molecular magnet ~ -d interaction metal-insulator transition spin ladder ferromagnet
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