Magnetic-circular-dichroism microspectroscopy at the spin reorientation transition in Ni(001) films

Abstract

The spin reorientation transition in fcc Co/Ni/Cu(001) epitaxial ultrathin films as a function of Co and Ni film thickness is studied by the combination of photoelectron emission microscopy and x-ray magnetic-circular-dichroism spectroscopy at the Ni ${L}_{2,3}$ edge. This microspectroscopic technique allows one to extract local quantitative information about the Ni magnetic properties on a submicrometer scale. Domain images in the thickness range of 1.4--2.6 atomic monolayers (ML) Co and 11--14 ML Ni show that the spin reorientation occurs as a function of both Co and Ni thicknesses. Increasing the Co thickness or decreasing the Ni thickness leads to a switching of the magnetic easy axis from $[001]$ out-of-plane to $〈110〉$ in-plane directions. A constant effective Ni spin moment similar to the bulk magnetic moment is observed. The Ni orbital to spin moment ratio shows distinctly different values for out-of-plane magnetization $(0.080\ifmmode\pm\else\textpm\fi{}0.005)$ and in-plane magnetization $(0.053\ifmmode\pm\else\textpm\fi{}0.005).$ This is discussed in terms of the connection to the Ni magnetocrystalline anisotropy. The domain density of the perpendicular magnetization increases towards the spin reorientation transition line.