Abstract
Co2FexMn1−xSi (0 ≦̸ x ≦̸ 1) Heusler alloys were fabricated by arc-melting the stoichiometric quantities of the constituents. We investigated the magnetic properties, geometric structure simulation, and real crystal structure for powder samples and the magnetic damping constant for polished thin-disk samples. All samples show high Curie temperatures, and the molecular magnetic moment increases with Fe concentration. The theoretical atomic site occupation of Co2FexMn1−xSi Heusler alloys with A2, B2, and L21 structures were simulated by Diamond 3.2. The real crystal structure was studied via x-ray diffraction measurement, followed by both Rietveld refinement and 57Fe Mössbauer spectroscopy. The result indicates that in addition to the main phase of L21, some B2 phases coexist in the samples, which will decrease the gap at the Fermi level and destroy half metallicity. The corresponding magnetic damping constant, deduced from the ferromagnetic resonance, decreases as the concentration of the L21 phase increases. Therefore, the ordered L21 structure is the key factor for improving the half metallicity and decreasing the magnetic damping constant. The results suggest that the Co2Fe0.7Mn0.3Si Heusler alloy with a 100% L21 phase is more suitable for applications.
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