Abstract
Magnetic properties of polycrystalline samples of Li 2TbF 6 were studied in high continuous magnetic fields up to 20 Teslas between 1.4 and 300 K. In this new structural type, all the results agree with the calculated Tb 4+ free ion values ( 8S 7 2 ground state multiplet), and the 4+ oxidation state of the terbium ion was unambiguously inferred. The particular crystal chemical behavior of the Tb 4+ ion is discussed using the phase relationship within the series of Li 2 M IVF 6 compounds.
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