Abstract

Magnetic properties of the spin density wave (SDW) phase in (TMTSF) 2 X (X=AsF 6 , PF 6 ) and (TMTTF) 2 Br were investigated through analyses of 1 H-NMR and static magnetization measurements. A divergent peak was observed, at the temperature T * well below the SDW transition temperature, in the 1 H spin-lattice relaxation rate in the incommensurate SDW phase of (TMTSF) 2 X. A decrease of the differential magnetic susceptibility of (TMTSF) 2 X with the field parallel to the a-axis was observed around T * . This anomaly indicates a difference of the spin canting above and below T * which divides the SDW phase. In the measurements of magnetic susceptibility on the commensurate SDW phase of (TMTTF) 2 Br, a large decrease of the spin susceptibility was observed above T SDW and non-activated type behavior in the b'-axis susceptibility is observed below the spin-flop field at low temperature. The data are discussed on the basis of commensurability.

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