Abstract

The magnetic properties of a diluted ferrimagnetic spinels system CoFe2–2xCr2xO4 are studied using the high-temperature series expansions method in the range 0 ≤ x ≤ 1. The inter-sublattice exchange interactions (JCo Cr or JCo–Fe) are calculated using the probability law. The high-temperature series expansions, together with the Padé-approximants method, are applied to the spinels systems CoFe2–2xCr2xO4 to determine the magnetic phase diagram, i.e., TC versus dilution x. The critical exponent associated with the magnetic susceptibility (γ) is deduced. PACS Nos.: 75.30.Et; 75.40.Cx; 74.25.Ha, 75.30.Cr

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