Abstract
Abstract The magnetic properties of TCNQ anion salts with polycations containing sulfur atoms in the main chain were investigated using ESR and magnetostatic methods. For the majority of these complex salts asymmetric ESR lines were recorded and characterized by g⊥, g∥, and ΔHmax values as well as by an asymmetry parameter δ′. An analysis of symmetrical ESR lines was carried out by the linear anamorphose technique. The temperature dependence of magnetic susceptibility χp was studied for the Ks [x, y] complex salts obtained. A correlation was found between the magnetic properties (ΔHmax, δ′, and χp) and the electrical properties ([sgrave]25, Ea) studied in our previous works.
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