Abstract

Magnetization measurements on chromic sulfide bromide were realized in the temperature range from 1.3 to 200 K in applied fields of up to 2 T. Below T N = 132 K, the substance orders as a two-sublattice antiferromagnet with anisotropic Heisenberg interaction. The magnetic phase diagram for fields parallel to the three orthorhombic crystal axes is determined. In the ordering direction no spin-flop phase exists. Mean-field calculations lead to good agreement with the observed magnetic behaviour.

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