Abstract

ABSTRACTThe magnetic properties and magnetic structures of Nd2TGe6 (T = Ni and Cu) were studied by magnetometric and neutron diffraction measurements. Both compounds have an orthorhombic crystal structure of the Ce2CuGe6-type and are antiferromagnetic with the Néel temperatures of 6.4 K (Nd2NiGe6) and 9.8 K (Nd2CuGe6). Based on the neutron diffraction data the magnetic structures were determined. In the investigated compounds all magnetic moments are localized on the Nd atoms and form a collinear commensurate magnetic structure with the magnetic unit cell equal to the crystal one. The moments are parallel to the b-axis (T = Ni) or to the c-axis (T = Cu). The obtained magnetic structures are discussed on the basis of competition between the RKKY-type interactions and influence of Crystalline Electric Field (CEF).

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