Abstract
Among six BETS (=bis(ethylenedithio)tetraselenafulvalene) superconductors, the systems with FeX 4 m (X=Cl, Br) anions exhibit salient electronic properties due to the coupling between ~ and d electron systems. u -BETS 2 FeCl 4 undergoes successive transitions as, antiferromagnetic insulating phase M metallic phase with ferromagnetically oriented Fe 3+ spins M superconducting phase ( H //conduction plane) M metallic phase, with increasing magnetic field. s -BETS 2 FeX 4 exhibits successive antiferromagnetic and superconducting transitions with decreasing temperature. Resistivity anomaly observed at antiferromagnetic transition temperature indicates an evidence for the coupling between ~ and d electron systems. antiferromagnetic organic superconductor BETS magnetic organic superconductor organic superconductor
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