Abstract

We report tuning of the moduli and surface roughness of magnetorheological elastomers (MREs) by varying applied magnetic field. Ultrasoft MREs are fabricated using a physiologically relevant commercial polymer, SylgardTM 527, and carbonyl iron powder (CIP). We found that the shear storage modulus, Young’s modulus, and root-mean-square surface roughness are increased by ∼41×, ∼11×, and ∼11×, respectively, when subjected to a magnetic field strength of 95.5 kA m−1. Single fit parameter equations are presented that capture the tunability of the moduli and surface roughness as a function of CIP volume fraction and magnetic field strength. These magnetic field-induced changes in the mechanical moduli and surface roughness of MREs are key parameters for biological applications.

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