Abstract

We investigate the ground state properties of the spin S=1 Kitaev honeycomb model under a magnetic field based on the density matrix renormalization group (DMRG) calculation. With the time reversal symmetry breaking due to the magnetic field, a gapped Kitaev spin liquid is identified for both ferromagnetic (FM) and antiferromagnetic (AFM) Kitaev couplings. The topological nature of such Kitaev spin liquid is manifested by the nearly quantized Wilson loop, degeneracy in the entanglement spectra and existence of edge modes. While the FM Kitaev spin liquid is destroyed by a weaker magnetic field $H_*^\text{FM}$, the AFM one demonstrates a robustness up to an order of magnitude larger critical field $H_*^\text{AFM}$. Moreover, an intermediate nonmagnetic phase appears only for the AFM case at larger fields, $H_*^\text{AFM} < H < H_{**}^\text{AFM}$, before the transition to a high-field polarized paramagnet. The stability of the Kitaev spin liquid against the Heisenberg interactions is also examined. Our findings may further inspire the investigation of recently proposed S=1 Kitaev materials.

Highlights

  • The search for exotic states of matter such as highly entangled quantum spin liquids (QSLs) has attracted considerable attention in the modern condensed matter field [1,2,3,4]

  • The realization of Kitaev physics in real materials has been proposed in transition metal oxides with strong spin-orbit coupling (SOC) and S = 1/2 local moments, in which the edge-sharing oxygen octahedra result in bond-dependent Ising interactions [6,7]

  • It is natural to ask if the perpendicular magnetic field can induce new QSLs in such real materials, which is distinct from the pure S = 1 Kitaev model [52,53,54,55,56,57] due to the lack of time-reversal symmetry [5]

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Summary

Rapid Communications

Zheng Zhu ,1,* Zheng-Yu Weng, and D. We investigate the ground state properties of the spin S = 1 Kitaev honeycomb model under a magnetic field based on the density matrix renormalization group (DMRG) calculation. With the time-reversal symmetry breaking due to the magnetic field, a gapped Kitaev spin liquid is identified for both ferromagnetic (FM) and antiferromagnetic (AFM) Kitaev couplings. While the FM Kitaev spin liquid is destroyed by a weaker magnetic field H∗FM, the AFM one demonstrates a robustness up to an order of magnitude larger critical field H∗AFM. An intermediate nonmagnetic phase appears only for the AFM case at larger fields, H∗AFM < H < H∗A∗FM, before the transition to a high-field polarized paramagnet. The stability of the Kitaev spin liquid against the Heisenberg interactions is examined.

Introduction
Published by the American Physical Society
FM KSL

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