Abstract

The magnetic properties of NO overlayers on a variety of ferromagnetic and paramagnetic (100) metal surfaces are calculated within the local-spin-density approximation. Bridge-site adsorption results in negligible spin densities in all cases on Rh, Pd, and Pt, and strongly suppresses the surface magnetic moments of Ni. Atop-site adsorption yields more complicated behavior, including residual NO magnetic moments on Pd (100) monolayers and induced ferromagnetism on thicker Pd and Pt slabs. \textcopyright{} 1996 The American Physical Society.

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