Magnetic and thermodynamic properties of mixed spin-3/2 and spin-3 Ising ferrimagnets on a 2D triangular lattice: Monte Carlo study

Abstract

Monte Carlo methods in the presence and absence of an external magnetic field were used to investigate the thermodynamic and magnetic properties of the mixed spins (3/2, 3) Ising ferrimagnets in a 2D triangular lattice consisting of sublattices A, B, and C. Two types of mixing were considered: S→=(SA,SB,SC)=(3/2,3,3) (Model I) and S→=(SA,SB,SC)=(3/2,3,3/2) (Model II). In contrast to bipartite lattices, the antiferromagnetic coupling between spin-3/2 and spin-3 in the triangular lattice leads to geometric frustrations that impact magnetic properties. Determination of ground state phase diagrams, combined with verification of whether or not there was magnetic hysteresis when crossing each transition line, revealed first- and second-order phase transition lines, as well as multicritical points. The temperature investigation in the absence of an external magnetic field revealed rich magnetic properties such as 1st- and 2nd-order phase transitions, N- and L-type compensation points, tricritical points, and critical endpoints, as well as M-, P-, Q-, R- and S-type total magnetization behaviours. The effect of the crystal field on finite-temperature phase diagrams and compensation behaviour was also carried out. As a result, the critical temperatures of Model II become constant when the crystal field is sufficiently strong. In contrast, several critical values of the crystal field for which the critical temperature is zero were identified for Model I. In the presence of a magnetic field, hysteresis behaviour and associated magnetic properties such as coercivity and magnetic remanence were investigated. The effect of crystal field and temperature was explored. Hysteresis of one to four loops were found at low temperatures when the crystal field varied. Finally, as the temperature rises, the hysteresis loops' area decreases to zero at high temperatures.