Abstract

Greenhouse gas (GHG) emissions from open-pit mines pose a global climate challenge, which necessitates appropriate quantification to support effective mitigation measures. This study considers the area-fugitive methane advective flux (as a proxy for emission flux) released from a tailings pond and two open-pit mines, denominated “old” and “new”, within a facility in northern Canada. To estimate the emission fluxes of methane from these sources, this research employed near-surface observations and modeling using the weather research and forecasting (WRF) passive tracer dispersion method. Various machine learning (ML) methods were trained and tested on these data for the operational forecasting of emissions. Predicted emission fluxes and meteorological variables from the WRF model were used as training and input datasets for ML algorithms. A series of 10 ML algorithms were evaluated. The four models that generated the most accurate forecasts were selected. These ML models are the multi-layer perception (MLP) artificial neural network, the gradient boosting (GBR), XGBOOST (XGB), and support vector machines (SVM). Overall, the simulations predicted the emission fluxes with R2 (-) values higher than 0.8 (-). Considering the bias (Tonnes h−1), the ML predicted the emission fluxes within 6.3%, 3.3%, and 0.3% of WRF predictions for the old mine, new mine, and the pond, respectively.

Highlights

  • In developed and developing countries, energy is a critical component supporting the development of the economy and society [1]

  • Mine activities often create large amounts of fugitive dust, odorous compounds, and greenhouse gas (GHG) [29], and the flow circulations, shear layers, and plume meandering created by mine pits [30] impact the transport of materials to downwind environments

  • The pond shows greater variability in the wind speed, surface heat flux, and emission flux noticed by the peaks from Figure 3a,c,d

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Summary

Introduction

In developed and developing countries, energy is a critical component supporting the development of the economy and society [1]. In the United States, more than 25% of the methane emitted into the atmosphere is a result of the oil and gas industry. Abating such emissions from the oil and gas sector is a critical component of mitigating climate change [3,4,5]. Methane has a global warming potential (GWP) 28 times greater than carbon dioxide for a duration of 100 years. One quarter of total global warming is related to the methane emissions from natural and anthropogenic sources. The short-term warming trends are affected by the methane lifetime, which is approximately 10 years [8]

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