Abstract
Based on a specially created theoretical model, frequency dependences of the luminescence intensity of the two-component “exciton-activated semiconductor quantum dot (QD)–plasmon nanoparticle (NP)” system in a constant magnetic field are calculated. In contrast to previous models, it goes beyond the scope of the approximation of dipole polarizability of a spherical NP. The induced NP dipole moment was calculated taking into account the inhomogeneous character of the field created by the QD containing an exciton. It is shown that, with a change in induction of the external magnetic field, one can observe transformation of exciton luminescence spectra of such system as a result of the exciton–plasmon interaction between cluster particles and magnetization of the NP electron plasma. The competition of radiative and nonradiative decay channels of the excited state of a two-particle complex is taken into account. It is shown that, in rate spectra of the nonradiative energy transfer from the QD to the NP, as well as of spontaneous emission of the nanocomplex, stripes of higher order multipole transitions are formed in addition to dipole stripes; they are split into doublet components in the magnetic field.
Published Version
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